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Definition of exasperatedly adverb from the Oxford Advanced Learner's Dictionary

exasperatedly

adverb

/ɪɡˈzæspəreɪtɪdli/,

/ɪɡˈzɑːspəreɪtɪdli/

/ɪɡˈzæspəreɪtɪdli/

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in an extremely annoyed way, especially because you cannot do anything to improve a situation
Oxford Collocations Dictionary
Exasperatedly is used with these verbs:
sigh
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